Which of the following is NOT a benefit of Permission Sets?

The choice identified as the correct answer highlights that limitations for the entire organization do not align with the primary benefits of Permission Sets. Permission Sets are designed to grant users additional access to various Salesforce features and data without altering their their profile settings. This means they offer specific access tailored to individual users or groups, which supports the first benefit.

When considering flexible sharing settings, Permission Sets provide a dynamic way to broaden access for users as needed, without requiring a complete reassessment of all organizational settings. This flexibility allows administrators to adjust permissions on a user-by-user basis, accommodating unique role requirements within different teams.

The ability to grant additional access is a core function of Permission Sets. They serve as a powerful tool for expanding user capabilities, making it easier to manage permissions across a diverse and scalable user base. This ensures that users receive the level of access suitable for their roles, without the need to create multiple profiles for different access levels.

In contrast, the idea of imposing limitations on the entire organization does not fit the structure or function of Permission Sets, as these are specifically intended to augment system access selectively rather than restrict it broadly across all users.